e-Assignment #3

Purpose & Results of the Free Radical Chlorination of 1-Chlorobutane

Purpose:

    The purpose of this laboratory experiment is to determine the relative reactivity of the different types of hydrogen atoms present on a 1-halogenated hydrocarbon.  In particular, the experiment will focus on the relative amount of each of the four dichlorinated products produced from the free radical chlorination of 1-chlorobutane.  By comparison of each product's percent composition as well as its statistical factor, the relative reactivity of the various hydrogen atoms in the starting material will be determined.
    The main chemical concepts being investigated during the experiment is free radical chlorination.  During free radical chlorination, a chlorine atom has the option of abstracting a primary hydrogen from the methyl group or a secondary hydrogen from one of the methylene groups to form a carbon radical on the carbon chain.  Typically, a secondary hydrogen will be more reactive and easier to abstract than a primary hydrogen; however, this assumption is not valid in the case of 1-chlorobutane because the affect due to the presence of the chlorine substituent is not known.  Analysis of the dichlorinated products will be carried out by gas chromatography and will hopefully provide insight into the effect a chlorine and its location can have on the relative reactivity of the hydrogen atoms in the molecule. 

Results:

peak areas

relative reactivities

Conclusions:

    It is apparent from the experiment’s results that 1,3-dichlorobutane is more readily produced from the starting material, which indicates more reactive hydrogen atoms on the third carbon in 1-chlorobutane.  In particular, the 1,3-dichlorobutane is 8 times more likely to be produced then the 1,1-dichlorobutane.  Typically, primary hydrogen atoms are not as reactive as secondary hydrogen atoms.  However, this trend is not followed explicitly due to the chlorine substituent on the starting material.  The presence of the chlorine substituent limits the amount of 1,1-dichlorbutane produced.  Steric hindrance interferes with the formation of a second C-Cl bond on the first carbon drastically.  It also plays a role in the formation of 1,2-dichlorobutane, but is less likely to affect the formation of the C-Cl bond on the third and fourth carbons.  This reasoning would indicate a higher percentage of the 1,4-dichlorobutane product than the 1,2-dichlorobutane; however, this is not evident in the gas chromatogram.  Therefore, there must be another factor in determining the relative reactivity of the hydrogen atoms  The last factor is most likely the stability of the carbon radical that forms during the free-radical process.  A radical will be more stable when there are more R groups attached to the carbon it is on.  The 1,4 product requires are radical to be present on the last carbon atom in the chain, which will be less stable than a radical present on the second carbon in the chain.  This is why the 1,2-dichlorobutane is more readily produced when compared to the 1,4-dichlorobutane.

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